题名 | 3D charge and 2D phonon transports leading to high out-of-plane ZT in n-type SnSe crystals |
作者 | |
通讯作者 | He, Jiaqing; Zhao, Li-Dong |
发表日期 | 2018-05-18
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DOI | |
发表期刊 | |
ISSN | 0036-8075
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EISSN | 1095-9203
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卷号 | 360期号:6390页码:778-782 |
摘要 | Thermoelectric technology enables the harvest of waste heat and its direct conversion into electricity. The conversion efficiency is determined by the materials figure of merit ZT. Here we show a maximum ZT of similar to 2.8 +/- 0.5 at 773 kelvin in n-type tin selenide (SnSe) crystals out of plane. The thermal conductivity in layered SnSe crystals is the lowest in the out-of-plane direction [two-dimensional (2D) phonon transport]. We doped SnSe with bromine to make n-type SnSe crystals with the overlapping interlayer charge density (3D charge transport). A continuous phase transition increases the symmetry and diverges two converged conduction bands. These two factors improve carrier mobility, while preserving a large Seebeck coefficient. Our findings can be applied in 2D layered materials and provide a new strategy to enhance out-of-plane electrical transport properties without degrading thermal properties. |
相关链接 | [来源记录] |
收录类别 | |
语种 | 英语
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重要成果 | NI期刊
; NI论文
; ESI高被引
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学校署名 | 通讯
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资助项目 | Early Career Scheme of the Research Grants Council[27202516]
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WOS研究方向 | Science & Technology - Other Topics
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WOS类目 | Multidisciplinary Sciences
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WOS记录号 | WOS:000432473500046
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出版者 | |
ESI学科分类 | BIOLOGY & BIOCHEMISTRY;CLINICAL MEDICINE;MULTIDISCIPLINARY;PLANT & ANIMAL SCIENCE;ENVIRONMENT/ECOLOGY;SOCIAL SCIENCES, GENERAL;MICROBIOLOGY;ECONOMICS BUSINESS;IMMUNOLOGY;MATERIALS SCIENCE;MATHEMATICS;COMPUTER SCIENCE;SPACE SCIENCE;MOLECULAR BIOLOGY & GENETICS;CHEMISTRY;PSYCHIATRY/PSYCHOLOGY;NEUROSCIENCE & BEHAVIOR;PHYSICS;GEOSCIENCES;ENGINEERING
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来源库 | Web of Science
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引用统计 |
被引频次[WOS]:866
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成果类型 | 期刊论文 |
条目标识符 | http://kc.sustech.edu.cn/handle/2SGJ60CL/27708 |
专题 | 理学院_物理系 |
作者单位 | 1.Beihang Univ, Sch Mat Sci & Engn, Beijing 100191, Peoples R China 2.Southern Univ Sci & Technol, Dept Phys, Shenzhen 518055, Peoples R China 3.Tsinghua Univ, Sch Mat Sci & Engn, Key Lab New Ceram & Fine Proc, Beijing 100084, Peoples R China 4.Univ Hong Kong, Dept Mech Engn, Hong Kong, Hong Kong, Peoples R China 5.Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201204, Peoples R China |
通讯作者单位 | 物理系 |
推荐引用方式 GB/T 7714 |
Chang, Cheng,Wu, Minghui,He, Dongsheng,et al. 3D charge and 2D phonon transports leading to high out-of-plane ZT in n-type SnSe crystals[J]. SCIENCE,2018,360(6390):778-782.
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APA |
Chang, Cheng.,Wu, Minghui.,He, Dongsheng.,Pei, Yanling.,Wu, Chao-Feng.,...&Zhao, Li-Dong.(2018).3D charge and 2D phonon transports leading to high out-of-plane ZT in n-type SnSe crystals.SCIENCE,360(6390),778-782.
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MLA |
Chang, Cheng,et al."3D charge and 2D phonon transports leading to high out-of-plane ZT in n-type SnSe crystals".SCIENCE 360.6390(2018):778-782.
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条目包含的文件 | ||||||
文件名称/大小 | 文献类型 | 版本类型 | 开放类型 | 使用许可 | 操作 | |
2018_Science_C_Chang(1228KB) | 期刊论文 | 作者接受稿 | 限制开放 | CC BY-NC-SA |
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