中文版 | English
题名

Functionalised heterogeneous catalysts for sustainable biomass valorisation

作者
通讯作者Sudarsanam, Putla; Parvulescu, Vasile I.; Sels, Bert F.
发表日期
2018-11-21
DOI
发表期刊
ISSN
0306-0012
EISSN
1460-4744
卷号47期号:22页码:8349-8402
摘要

Efficient transformation of biomass to value-added chemicals and high-energy density fuels is pivotal for a more sustainable economy and carbon-neutral society. In this framework, developing potential cascade chemical processes using functionalised heterogeneous catalysts is essential because of their versatile roles towards viable biomass valorisation. Advances in materials science and catalysis have provided several innovative strategies for the design of new appealing catalytic materials with well-defined structures and special characteristics. Promising catalytic materials that have paved the way for exciting scientific breakthroughs in biomass upgrading are carbon materials, metal-organic frameworks, solid phase ionic liquids, and magnetic iron oxides. These fascinating catalysts offer unique possibilities to accommodate adequate amounts of acid-base and redox functional species, hence enabling various biomass conversion reactions in a one-pot way. This review therefore aims to provide a comprehensive account of the most significant advances in the development of functionalised heterogeneous catalysts for efficient biomass upgrading. In addition, this review highlights important progress ensued in tailoring the immobilisation of desirable functional groups on particular sites of the above-listed materials, while critically discussing the role of consequent properties on cascade reactions as well as on other vital processes within the bio-refinery. Current challenges and future opportunities towards a rational design of novel functionalised heterogeneous catalysts for sustainable biomass valorisation are also emphasized.

相关链接[来源记录]
收录类别
语种
英语
重要成果
ESI高被引
学校署名
其他
资助项目
UEFISCDI[PN-III-P4-ID-PCE-2016-0146] ; UEFISCDI[32PCCDI-2018]
WOS研究方向
Chemistry
WOS类目
Chemistry, Multidisciplinary
WOS记录号
WOS:000449968700006
出版者
ESI学科分类
CHEMISTRY
来源库
Web of Science
引用统计
被引频次[WOS]:436
成果类型期刊论文
条目标识符http://kc.sustech.edu.cn/handle/2SGJ60CL/26940
专题理学院_化学系
作者单位
1.Katholieke Univ Leuven, Fac Biosci Engn, Ctr Surface Chem & Catalysis, Celestijnenlaan 200f, B-3001 Heverlee, Belgium
2.Southern Univ Sci & Technol, Dept Chem, Shenzhen 518055, Peoples R China
3.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
4.Univ Bucharest, Dept Organ Chem Biochem & Catalysis, Bdul Regina Elisabeta 4-12, Bucharest 030016, Romania
推荐引用方式
GB/T 7714
Sudarsanam, Putla,Zhong, Ruyi,Van den Bosch, Sander,et al. Functionalised heterogeneous catalysts for sustainable biomass valorisation[J]. CHEMICAL SOCIETY REVIEWS,2018,47(22):8349-8402.
APA
Sudarsanam, Putla,Zhong, Ruyi,Van den Bosch, Sander,Coman, Simona M.,Parvulescu, Vasile I.,&Sels, Bert F..(2018).Functionalised heterogeneous catalysts for sustainable biomass valorisation.CHEMICAL SOCIETY REVIEWS,47(22),8349-8402.
MLA
Sudarsanam, Putla,et al."Functionalised heterogeneous catalysts for sustainable biomass valorisation".CHEMICAL SOCIETY REVIEWS 47.22(2018):8349-8402.
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